Abstract/Details

A gas injection negative ion source for accelerator mass spectrometry


2004 2004

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Abstract (summary)

Accelerator mass spectrometry is an ultra-sensitive isotopic analysis technique that allows for the determination of rare long-lived radionuclides such as radiocarbon. Historically, the technique has required that samples be processed into graphite prior to analysis. The processing is time and labor intensive and limits the technique due to contamination. There has been recent interest to develop an ion source that would allow direct injection of gaseous samples, thus eliminating the processing. Previous attempts to build such an ion source have been limited by low mass usage efficiency and severe memory effects. This dissertation describes the development of a plasma negative ion source that allows direct injection of gaseous material. This ion source was able to produce a 12C ion beam of approximately 4.5 μA from carbon dioxide. This beam intensity is lower than both of the competing designs. However, this ion source was able to operate with a mass efficiency of nearly 0.15% which exceeds one of the competing designs. It was also free from significant memory effects which plagued the other competing design. There are many improvements to the design of this ion source that would further enhance its performance. These results are promising and show that this type of ion source could be used effectively in an accelerator mass spectrometry system.

Indexing (details)


Subject
Nuclear chemistry
Classification
0738: Nuclear chemistry
Identifier / keyword
Pure sciences; Accelerator mass spectrometry; Gas injection; Ion source
Title
A gas injection negative ion source for accelerator mass spectrometry
Author
Tumey, Scott Joseph
Number of pages
130
Publication year
2004
Degree date
2004
School code
0117
Source
DAI-B 65/11, Dissertation Abstracts International
Place of publication
Ann Arbor
Country of publication
United States
ISBN
049612773X, 9780496127733
Advisor
Mignerey, Alice C.
University/institution
University of Maryland, College Park
University location
United States -- Maryland
Degree
Ph.D.
Source type
Dissertations & Theses
Language
English
Document type
Dissertation/Thesis
Dissertation/thesis number
3152508
ProQuest document ID
305175679
Copyright
Database copyright ProQuest LLC; ProQuest does not claim copyright in the individual underlying works.
Document URL
http://search.proquest.com/docview/305175679
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